Etymology
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unsettle (v.)

1590s, "undo from a fixed position," from un- (2) "reverse, opposite of" + settle (v.). Of the mind, feelings, etc., attested from 1640s. Related: Unsettled; unsettling.

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Definitions of unsettle

unsettle (v.)
disturb the composure of;
Synonyms: faze / unnerve / enervate
From wordnet.princeton.edu