1520s, "marked by misfortune or failure," from un- (1) "not" + lucky (adj.). Similar formation in West Frisian unlokkich, Mliddle Low German unluckich. Sense of "boding ill" is recorded from 1540s; that of "having bad luck" is from 1550s; that of "bringing bad luck" is from 1580s. Related: Unluckily; unluckiness.
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