Etymology
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chunk (n.)

"short, thick piece" of something, 1690s, probably a nasalized variant of chuck (n.1) "cut of meat;" meaning "large amount" is 1883, American English. Meaning "person or beast that is small but thick-set and strong" is from 1822.

chunk (v.)

"to throw," 1835, American English, from chunk (n.) or by similar mutation from chuck (v.1). Related: Chunked; chunking.

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Definitions of chunk
1
chunk (v.)
put together indiscriminately;
Synonyms: lump
chunk (v.)
group or chunk together in a certain order or place side by side;
Synonyms: collocate / lump
2
chunk (n.)
a compact mass;
Synonyms: ball / clod / glob / lump / clump
chunk (n.)
a substantial amount;
we won a chunk of money
From wordnet.princeton.edu