Etymology
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adamant (adj.)

late 14c., "hard, unbreakable," from adamant (n.). The figurative sense of "unshakeable" (in belief, etc.) is by 1670s. Related: Adamantly; adamance.

adamant (n.)

"a very hard stone," mid-14c., adamant, adamaunt, from Old French adamant "diamond; magnet" or directly from Latin adamantem (nominative adamas) "adamant, hardest iron, steel," also used figuratively, of character, from Greek adamas (genitive adamantos), the name of a hypothetical hardest material.

It is a noun use of an adjective meaning "unbreakable, inflexible," which was metaphoric of anything unalterable (such as Hades) and is of uncertain origin. It is perhaps literally "invincible, indomitable," from a- "not" (see a- (3)) + daman "to conquer, to tame," from PIE root *deme- "to constrain, force, break (horses)," for which see tame (adj.). "But semantically, the etymology is rather strange," according to Beekes, who suggests it might be a foreign word altered in Greek by folk etymology, and compares Akkadian (Semitic) adamu.

Applied in antiquity to a metal resembling gold (Plato), white sapphire (Pliny), magnet (Ovid, perhaps through confusion with Latin adamare "to love passionately"), steel, emery stone, and especially diamond, which is a variant of this word. "The name has thus always been of indefinite and fluctuating sense" [Century Dictionary]. The word had been in Old English as aðamans, but the modern word is a re-borrowing.

updated on September 14, 2022

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Definitions of adamant from WordNet
1
adamant (n.)
very hard native crystalline carbon valued as a gem;
Synonyms: diamond
2
adamant (adj.)
impervious to pleas, persuasion, requests, reason; "Cynthia was inexorable; she would have none of him"- W.Churchill;
he is adamant in his refusal to change his mind
Etymologies are not definitions. From wordnet.princeton.edu, not affiliated with etymonline.